Šimunović started his career as a journalist at Večernji List, a conservative daily newspaper in Zagreb, from 1988 to 1990. He covered the unraveling of the Soviet empire in Eastern Europe, including free elections in Poland, the Romanian Revolution, the fall of the Berlin Wall, and other events. He later served as national coordinator for NATO, as well as assistant minister for International Organizations and Security, from 2004 to 2008, and as ambassador to Israel from 2012 to 2016.
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